Description
Meteorites provide an opportunity to reconstruct the history of the SolarSystem. Differentiated meteorites, also called achondrites, are the result of melting
and differentiation processes on their parent body. Stable isotopic compositions of
differentiated meteorites and their components have added to the understanding of
physical parameters, such as temperature, pressure, and redox conditions relevant
to differentiation processes on planetesimals and planets in the early Solar System.
In particular, Fe and Si isotopes have proven to be useful in advancing the
understanding of physical and chemical processes during planetary accretion and
subsequent evolution.
In this work, I developed a new method to simultaneously purify Fe and Si
from a single aliquot of sample while ensuring consistently high yields and accurate
and precise isotopic measurements. I then measured the Fe isotope compositions
and Si contents of metals from aubrite meteorites to infer the structure and thermal
evolution of their asteroidal parent body. Thereafter, I determined the combined Si
and Fe isotope compositions of aubrite metals and the Horse Creek iron meteorite,
and compared the magnitude of Si and Fe isotope fractionation factors between
metal and silicates for both enstatite chondrites and aubrites to estimate the effect of
high-temperature core formation that occurred on the aubrite parent body. I
additionally assessed whether correlated Si and Fe isotope systematics can be used
to trace core formation and partial melting processes for the aubrite parent body,
angrite parent body, Mars, Vesta, Moon, and Earth. Finally, I measured the combined
Fe and Si isotope composition of a variety of ungrouped achondrites and brachinites
that record different degrees of differentiation under different redox conditions to
evaluate the role of differentiation and oxygen fugacity in controlling their Fe and Si
isotope compositions. Taken together, this comprehensive dataset reveals the
thermal evolution of the aubrite parent body, provides insights into the factors controlling the Fe and Si isotope compositions of various planetary materials, and
helps constrain the bulk starting composition of planets and planetesimals.
Download count: 1
Details
Title
- A Combined Investigation of Iron and Silicon Isotopes in Meteorites: Implications for Planetary Accretion and Differentiation
Contributors
- Ray, Soumya (Author)
- Wadhwa, Meenakshi (Thesis advisor)
- Garvie, Laurence (Committee member)
- Till, Christy (Committee member)
- Hervig, Richard (Committee member)
- Schrader, Devin (Committee member)
- Arizona State University (Publisher)
Date Created
The date the item was original created (prior to any relationship with the ASU Digital Repositories.)
2021
Subjects
Resource Type
Collections this item is in
Note
- Partial requirement for: Ph.D., Arizona State University, 2021
- Field of study: Geological Sciences